A Comprehensive Treatise Inorganic and Theoretical Chemistry by Mellor J.W. PDF

By Mellor J.W.

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Soc. Lond. A (1993) On the formation of the fullerenes 27 Quantum theoretical calculations by Scuseria's group (Strout et al. 1992) show that napthalenic C10 is much higher in energy than simple C10 rings (ring I). This seems fatal for the model because no matter how reactive a species is, any pathway where it reacts with itself will be minor unless the concentration of the species is high. The other model of C^0F formation building up from intermediate size clusters has been proposed by Wakabayashi & Achiba (1992).

The other model of C^0F formation building up from intermediate size clusters has been proposed by Wakabayashi & Achiba (1992). In this mechanism napthalenic Clo combines with ring C18 to form a building block ' open' fullerene C28 well on the path to C60. ) As mentioned above, it is unlikely that napthalenic C10 can ever be present in significant amounts. However, the Scuseria group calculations (Strout et al. 1992) suggest that when ring C10 is placed inside a C18 ring, it begins to distort in the direction of producing the appropriate C28 intermediate.

We still could not completely exclude the possibility that the ra lines were produced by contaminant, and we felt that such a sensational result, if true, had to be substantiated by additional experiments. 4. Fullerites As part of his thesis work K. Fostiropoulos, in Heidelberg, investigated the effects of possible soot contamination and used much cleaner conditions and procedures than used previously. The appearance of the camel hump was not affected. With slightly renewed confidence we presented a paper of this observation at a workshop on interstellear matter in September 1989 (Kratschmer et al.

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A Comprehensive Treatise Inorganic and Theoretical Chemistry by Mellor J.W.


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